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Hypothetically, could, say Darkseid, Lex Luthor or even Dr Doom (individually) have obtained the complete set of Infinity gems from their original guardians? Are they smart or cunning enough?

Time - Gardener
Space - Runner
Reality - Collector
Power - Champion
Soul - In Betweener
Mind - Grandmaster

Well i think it would be a bit hard for Darkseid or Lex Luther coz there in different universes. And i doubt Dr.Doom could have.

Doom or Darkseid could. The Guardians aren't exactly genius.

Krissy Von Doom was a sock

Soul and power are pretty hard to get a hold of.

i feel dr doom could have done it. darkseid would have tried but i dont see him pulling it off.

Darkseid could actually beat a handful of them, so he should be able to get a couple. If he went for the in-betweener and runner last he could make it.