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Can Longshot make the impossible shot to kill Deadpool?

No, but he can KO him.

Can Deadshot take the shot from beyond the 4th Wall with rubber eraser bullets?

I was thinking that if Longshot caught the wind like he did to carry the X-men against the Advisory near a Volcano in Hawaii and Deadpool is near the Volcano Longshot could get lucky and the Volcano could erupt and Longshot could throw 4 darts in the shape of + at Deadpool and cut him into 4.