I would say ROTS Anakin at the beginning. Although it may appear like he was more aggressive as a sith, Anakin as a Jedi was more stable. Before he started worrying about his wife dying, he had nothing to look back to, it was as if the future was in front of him until that stuff started. I would say Anakin at the beginning.
Yeah, definitly jedi knight anakin. I believe that while a jedi, anakin was much more focus and somehow less cocky, knowing how to concentrate his powers and even his emotions in an enemy, like he did against dooku. So, I basicly think that by turning to the darkside, anakin lost the switch to turn "Anakin in teh zone" on, lol.