Meh. Thor in Hulk vs. was a bigtime pussy. Hulk in Planet Hulk wasn't that great as well. I'd say:
Superman Unbound > Superman MOS
Thor movie > Thor (Hulk vs)
Incredible Hulk > Planet Hulk
Now if you use Hulk from Hulk vs. and Thor from EMH (or even just Ultimate Avengers), then we'd have the animations dominating.